BIBLIOS

Document type
Journal articles

Document subtype
Full paper

Title
Identifying imprints of externally derived dust and halogens in the sedimentary record of an Iberian alpine lake for the past ∼13,500 years – Lake Peixão, Serra da Estrela (Central Portugal)

Participants in the publication
J. Moreno (Author)
IDL
A.M. Ramos (Author)
IDL
P.M. Raposeiro (Author)
R.N. Santos (Author)
T. Rodrigues (Author)
F. Naughton (Author)
F. Moreno (Author)
R.M. Trigo (Author)
Instituto Dom Luiz (IDL), Faculdade de Ciências, Universidade de Lisboa, Campo Grande, 1749–016, Lisboa, Portugal
Dep. Engenharia Geográfica, Geofísica e Energia
J. Ibañez-Insa (Author)
P. Ludwig (Author)
X. Shi (Author)
A. Hernández (Author)

Summary
Iberian lacustrine sediments are a valuable archive to document environmental changes since the last glacial termination, seen as key for anticipating future climate/environmental changes and their far-reaching implications for generations to come. Herein, multi-proxy-based indicators of a mountain lake record from Serra da Estrela were used to reconstruct atmospheric (in)fluxes and associated climatic/environmental changes over the last ∼13.5 ka. Depositions of long-range transported dust (likely from the Sahara) and halogens (primarily derived from seawater) were higher for the pre-Holocene, particularly in the late Bølling-Allerød–Younger Dryas period, compared to the Holocene. This synchronous increase could be related to a recognized dust-laden atmosphere, along with the combined effect of (i) an earlier proposed effective transport of Sahara dust for higher latitudes during cold periods and (ii) the progressive Polar Front expansion southwards, with the amplification of halogen activation reactions in lower latitudes due to greater closeness to snow/sea ice (halide-laden) surfaces. Additionally, the orographic blocking of Serra da Estrela may have played a critical role in increasing precipitation of Atlantic origin at higher altitudes, with the presence of snow prompting physical and chemical processes involving halogen species. In the Late Holocene, the dust proxy records highlighted two periods of enhanced input to Lake Peixão, the first (∼3.5–2.7 ka BP) after the end of the last African Humid Period and the second, from the 19th century onwards, agreeing with the advent of commercial agriculture, and human contribution to land degradation and dust emission in the Sahara/Sahel region. The oceanic imprints throughout the Holocene matched well with North Atlantic rapid climatic changes that, in turn, coincided with ice-rafted debris or Bond events and other records of increased storminess for the European coasts. Positive parallel peaks in halogens were found in recent times, probably connected to fire extinction by halogenated alkanes and roadway de-icing.

Editor(s)
Sergi González-Herrero, Marc Lemus-Canovas, Paulo Pereira


Where published
Science of The Total Environment

Publication Identifiers
ISSN - 0048-9697

Publisher
Elsevier BV



Document Identifiers
DOI - https://doi.org/10.1016/j.scitotenv.2023.166179
URL - http://dx.doi.org/10.1016/j.scitotenv.2023.166179

Rankings
Web Of Science Q1 (2021) - 10.753 - ENVIRONMENTAL SCIENCES - SCIE